Tuning the activity of Pt alloy electrocatalysts by means of the lanthanide contraction.
Identifieur interne : 000006 ( Main/Exploration ); précédent : 000005; suivant : 000007Tuning the activity of Pt alloy electrocatalysts by means of the lanthanide contraction.
Auteurs : María Escudero-Escribano [États-Unis] ; Paolo Malacrida [Danemark] ; Martin H. Hansen [Danemark] ; Ulrik G. Vej-Hansen [Danemark] ; Amado Velázquez-Palenzuela [Danemark] ; Vladimir Tripkovic [Danemark] ; Jakob Schi Tz [Danemark] ; Jan Rossmeisl [Danemark] ; Ifan E L. Stephens [États-Unis] ; Ib Chorkendorff [Danemark]Source :
- Science (New York, N.Y.) [ 1095-9203 ] ; 2016.
Abstract
The high platinum loadings required to compensate for the slow kinetics of the oxygen reduction reaction (ORR) impede the widespread uptake of low-temperature fuel cells in automotive vehicles. We have studied the ORR on eight platinum (Pt)-lanthanide and Pt-alkaline earth electrodes, Pt5M, where M is lanthanum, cerium, samarium, gadolinium, terbium, dysprosium, thulium, or calcium. The materials are among the most active polycrystalline Pt-based catalysts reported, presenting activity enhancement by a factor of 3 to 6 over Pt. The active phase consists of a Pt overlayer formed by acid leaching. The ORR activity versus the bulk lattice parameter follows a high peaked "volcano" relation. We demonstrate how the lanthanide contraction can be used to control strain effects and tune the activity, stability, and reactivity of these materials.
DOI: 10.1126/science.aad8892
PubMed: 27034369
Affiliations:
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Hansen</name><affiliation wicri:level="1"><nlm:affiliation>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen</wicri:regionArea><placeName><settlement type="city">Copenhague</settlement><region type="région" nuts="2">Hovedstaden</region></placeName></affiliation></author><author><name sortKey="Vej Hansen, Ulrik G" sort="Vej Hansen, Ulrik G" uniqKey="Vej Hansen U" first="Ulrik G" last="Vej-Hansen">Ulrik G. Vej-Hansen</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. 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Department of Energy Conversion and Storage, Technical University of Denmark, 4000 Roskilde, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Energy Conversion and Storage, Technical University of Denmark, 4000 Roskilde</wicri:regionArea><wicri:noRegion>4000 Roskilde</wicri:noRegion></affiliation></author><author><name sortKey="Schi Tz, Jakob" sort="Schi Tz, Jakob" uniqKey="Schi Tz J" first="Jakob" last="Schi Tz">Jakob Schi Tz</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author><author><name sortKey="Rossmeisl, Jan" sort="Rossmeisl, Jan" uniqKey="Rossmeisl J" first="Jan" last="Rossmeisl">Jan Rossmeisl</name><affiliation wicri:level="1"><nlm:affiliation>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen</wicri:regionArea><placeName><settlement type="city">Copenhague</settlement><region type="région" nuts="2">Hovedstaden</region></placeName></affiliation></author><author><name sortKey="Stephens, Ifan E L" sort="Stephens, Ifan E L" uniqKey="Stephens I" first="Ifan E L" last="Stephens">Ifan E L. Stephens</name><affiliation wicri:level="2"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, USA. ibchork@fysik.dtu.dk ifan@fysik.dtu.dk maria.escudero@fysik.dtu.dk.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139</wicri:regionArea><placeName><region type="state">Massachusetts</region></placeName></affiliation></author><author><name sortKey="Chorkendorff, Ib" sort="Chorkendorff, Ib" uniqKey="Chorkendorff I" first="Ib" last="Chorkendorff">Ib Chorkendorff</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. ibchork@fysik.dtu.dk ifan@fysik.dtu.dk maria.escudero@fysik.dtu.dk.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2016">2016</date><idno type="doi">10.1126/science.aad8892</idno><idno type="RBID">pubmed:27034369</idno><idno type="pmid">27034369</idno><idno type="wicri:Area/PubMed/Corpus">000006</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">000006</idno><idno type="wicri:Area/PubMed/Curation">000006</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Curation">000006</idno><idno type="wicri:Area/PubMed/Checkpoint">000006</idno><idno type="wicri:explorRef" wicri:stream="Checkpoint" wicri:step="PubMed">000006</idno><idno type="wicri:Area/Ncbi/Merge">000B25</idno><idno type="wicri:Area/Ncbi/Curation">000B25</idno><idno type="wicri:Area/Ncbi/Checkpoint">000B25</idno><idno type="wicri:Area/Main/Merge">000006</idno><idno type="wicri:Area/Main/Curation">000006</idno><idno type="wicri:Area/Main/Exploration">000006</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Tuning the activity of Pt alloy electrocatalysts by means of the lanthanide contraction.</title><author><name sortKey="Escudero Escribano, Maria" sort="Escudero Escribano, Maria" uniqKey="Escudero Escribano M" first="María" last="Escudero-Escribano">María Escudero-Escribano</name><affiliation wicri:level="2"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Chemical Engineering, Stanford University, Stanford, CA 94305, USA. ibchork@fysik.dtu.dk ifan@fysik.dtu.dk maria.escudero@fysik.dtu.dk.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Chemical Engineering, Stanford University, Stanford, CA 94305</wicri:regionArea><placeName><region type="state">Californie</region></placeName></affiliation></author><author><name sortKey="Malacrida, Paolo" sort="Malacrida, Paolo" uniqKey="Malacrida P" first="Paolo" last="Malacrida">Paolo Malacrida</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author><author><name sortKey="Hansen, Martin H" sort="Hansen, Martin H" uniqKey="Hansen M" first="Martin H" last="Hansen">Martin H. Hansen</name><affiliation wicri:level="1"><nlm:affiliation>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen</wicri:regionArea><placeName><settlement type="city">Copenhague</settlement><region type="région" nuts="2">Hovedstaden</region></placeName></affiliation></author><author><name sortKey="Vej Hansen, Ulrik G" sort="Vej Hansen, Ulrik G" uniqKey="Vej Hansen U" first="Ulrik G" last="Vej-Hansen">Ulrik G. Vej-Hansen</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author><author><name sortKey="Velazquez Palenzuela, Amado" sort="Velazquez Palenzuela, Amado" uniqKey="Velazquez Palenzuela A" first="Amado" last="Velázquez-Palenzuela">Amado Velázquez-Palenzuela</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author><author><name sortKey="Tripkovic, Vladimir" sort="Tripkovic, Vladimir" uniqKey="Tripkovic V" first="Vladimir" last="Tripkovic">Vladimir Tripkovic</name><affiliation wicri:level="1"><nlm:affiliation>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Energy Conversion and Storage, Technical University of Denmark, 4000 Roskilde, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Energy Conversion and Storage, Technical University of Denmark, 4000 Roskilde</wicri:regionArea><wicri:noRegion>4000 Roskilde</wicri:noRegion></affiliation></author><author><name sortKey="Schi Tz, Jakob" sort="Schi Tz, Jakob" uniqKey="Schi Tz J" first="Jakob" last="Schi Tz">Jakob Schi Tz</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author><author><name sortKey="Rossmeisl, Jan" sort="Rossmeisl, Jan" uniqKey="Rossmeisl J" first="Jan" last="Rossmeisl">Jan Rossmeisl</name><affiliation wicri:level="1"><nlm:affiliation>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen, Denmark.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Atomic-Scale Materials Design (CAMD), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Nano-Science Center, Department of Chemistry, University of Copenhagen, 2100 Copenhagen</wicri:regionArea><placeName><settlement type="city">Copenhague</settlement><region type="région" nuts="2">Hovedstaden</region></placeName></affiliation></author><author><name sortKey="Stephens, Ifan E L" sort="Stephens, Ifan E L" uniqKey="Stephens I" first="Ifan E L" last="Stephens">Ifan E L. Stephens</name><affiliation wicri:level="2"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, USA. ibchork@fysik.dtu.dk ifan@fysik.dtu.dk maria.escudero@fysik.dtu.dk.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139</wicri:regionArea><placeName><region type="state">Massachusetts</region></placeName></affiliation></author><author><name sortKey="Chorkendorff, Ib" sort="Chorkendorff, Ib" uniqKey="Chorkendorff I" first="Ib" last="Chorkendorff">Ib Chorkendorff</name><affiliation wicri:level="1"><nlm:affiliation>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby, Denmark. ibchork@fysik.dtu.dk ifan@fysik.dtu.dk maria.escudero@fysik.dtu.dk.</nlm:affiliation><country xml:lang="fr">Danemark</country><wicri:regionArea>Center for Individual Nanoparticle Functionality (CINF), Department of Physics, Technical University of Denmark, 2800 Lyngby</wicri:regionArea><wicri:noRegion>2800 Lyngby</wicri:noRegion></affiliation></author></analytic><series><title level="j">Science (New York, N.Y.)</title><idno type="eISSN">1095-9203</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The high platinum loadings required to compensate for the slow kinetics of the oxygen reduction reaction (ORR) impede the widespread uptake of low-temperature fuel cells in automotive vehicles. We have studied the ORR on eight platinum (Pt)-lanthanide and Pt-alkaline earth electrodes, Pt5M, where M is lanthanum, cerium, samarium, gadolinium, terbium, dysprosium, thulium, or calcium. The materials are among the most active polycrystalline Pt-based catalysts reported, presenting activity enhancement by a factor of 3 to 6 over Pt. The active phase consists of a Pt overlayer formed by acid leaching. The ORR activity versus the bulk lattice parameter follows a high peaked "volcano" relation. We demonstrate how the lanthanide contraction can be used to control strain effects and tune the activity, stability, and reactivity of these materials.</div></front></TEI><affiliations><list><country><li>Danemark</li><li>États-Unis</li></country><region><li>Californie</li><li>Hovedstaden</li><li>Massachusetts</li></region><settlement><li>Copenhague</li></settlement></list><tree><country name="États-Unis"><region name="Californie"><name sortKey="Escudero Escribano, Maria" sort="Escudero Escribano, Maria" uniqKey="Escudero Escribano M" first="María" last="Escudero-Escribano">María Escudero-Escribano</name></region><name sortKey="Stephens, Ifan E L" sort="Stephens, Ifan E L" uniqKey="Stephens I" first="Ifan E L" last="Stephens">Ifan E L. Stephens</name></country><country name="Danemark"><noRegion><name sortKey="Malacrida, Paolo" sort="Malacrida, Paolo" uniqKey="Malacrida P" first="Paolo" last="Malacrida">Paolo Malacrida</name></noRegion><name sortKey="Chorkendorff, Ib" sort="Chorkendorff, Ib" uniqKey="Chorkendorff I" first="Ib" last="Chorkendorff">Ib Chorkendorff</name><name sortKey="Hansen, Martin H" sort="Hansen, Martin H" uniqKey="Hansen M" first="Martin H" last="Hansen">Martin H. Hansen</name><name sortKey="Rossmeisl, Jan" sort="Rossmeisl, Jan" uniqKey="Rossmeisl J" first="Jan" last="Rossmeisl">Jan Rossmeisl</name><name sortKey="Schi Tz, Jakob" sort="Schi Tz, Jakob" uniqKey="Schi Tz J" first="Jakob" last="Schi Tz">Jakob Schi Tz</name><name sortKey="Tripkovic, Vladimir" sort="Tripkovic, Vladimir" uniqKey="Tripkovic V" first="Vladimir" last="Tripkovic">Vladimir Tripkovic</name><name sortKey="Vej Hansen, Ulrik G" sort="Vej Hansen, Ulrik G" uniqKey="Vej Hansen U" first="Ulrik G" last="Vej-Hansen">Ulrik G. Vej-Hansen</name><name sortKey="Velazquez Palenzuela, Amado" sort="Velazquez Palenzuela, Amado" uniqKey="Velazquez Palenzuela A" first="Amado" last="Velázquez-Palenzuela">Amado Velázquez-Palenzuela</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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